NSUF 15-532: Atom probe tomography of Fe-U-Pu-Zr systems

Plutonium-uranium-zirconium (Pu-U-Zr) alloys have attracted attention for application in advanced fast reactors. Compatibility of the fuel with cladding is one of the most important factors that have to be considered prior to an alloy’s implementation in nuclear reactor environment. Interdiffusion between fuel and cladding is imperative for understanding of the useful lifetime of nuclear reactor components and fuels. The project aims to characterize complex phases formed upon heat treatment of diffusion couples constructed from Pu-U-Zr alloys and Fe cladding. Detailed chemical and structural characterization of interdiffusion between fuel and cladding the atomic scale is of profound consequence for evaluation of nuclear fuels and materials behavior. This proposal requests access to focused ion beam (FIB) and localized electrode atom probe (LEAP) instruments for thorough characterization of formed intermetallic phases. The proposed work will lead to enhancement of fundamental understanding of fuel performance and fuel-cladding chemical interactions.

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Abstract Plutonium-uranium-zirconium (Pu-U-Zr) alloys have attracted attention for application in advanced fast reactors. Compatibility of the fuel with cladding is one of the most important factors that have to be considered prior to an alloy’s implementation in nuclear reactor environment. Interdiffusion between fuel and cladding is imperative for understanding of the useful lifetime of nuclear reactor components and fuels. The project aims to characterize complex phases formed upon heat treatment of diffusion couples constructed from Pu-U-Zr alloys and Fe cladding. Detailed chemical and structural characterization of interdiffusion between fuel and cladding the atomic scale is of profound consequence for evaluation of nuclear fuels and materials behavior. This proposal requests access to focused ion beam (FIB) and localized electrode atom probe (LEAP) instruments for thorough characterization of formed intermetallic phases. The proposed work will lead to enhancement of fundamental understanding of fuel performance and fuel-cladding chemical interactions.
Award Announced Date 2014-12-04T00:00:00
Awarded Institution None
Facility None
Facility Tech Lead Yaqiao Wu
Irradiation Facility None
PI Assel Aitkaliyeva
PI Email [email protected]
Project Type RTE
RTE Number 532