NSUF 18-1484: EPMA Characterization of Actinide Redistribution and Fission Product Composition in MOX Fuels

The chemistry of MOX fuels and their secondary fission product phases can have significant impact on the thermal properties of the irradiated fuel. In order to predict the fuel response at varying fuel lifetimes, it is necessary to comprehensively understand the chemistry of the fuel and its constituent phases. This project aims to quantitatively determine the chemistry of irradiated MOX fuel pellets and early and end-of-life burnup conditions. Electron probe microanalysis (EPMA) will be performed to assess the radial concentration of U, Pu, and Am as a result of actinide redistribution and the chemical nature of secondary fission product phases. Once complete, this project will provide a thorough understanding of the chemical state of MOX fuels and their relevant phases that form during burnup. This information will have a significant impact on the understanding of MOX fuel evolution, with the potential to also aid in improving the accuracy of models used in predictive simulations.

Informazioni addizionali

Campo Valore
Awarded Institution University of Florida
Embargo End Date 2020-02-17
Facility Tech Lead Alina Montrose, Mukesh Bachhav
NSUF Call FY 2018 RTE 2nd Call
PI Casey McKinney
Project Member Dr. Jason Harp, Group Leader - Oak Ridge National Laboratory (https://orcid.org/0000-0002-5345-8440)
Project Member Professor Assel Aitkaliyeva, Assistant Professor - University of Florida (https://orcid.org/0000-0003-1481-6804)
Project Member Dr. Casey McKinney, Postdoctoral Research Associate - Oak Ridge National Laboratory (https://orcid.org/0000-0003-3538-3614)
Project Notes Awarded on 05/17/2018
Project Type RTE
Publication Characterization of solid fission products in 13.7% FIMA MOX fuel using electron microscopy techniques Riley Parrish, Karen Wright, Alexander Winston, Jason Harp, Casey McKinney, Assel Aitkaliyeva Journal of Nuclear Materials 524 2019-06-29 https://www.sciencedirect.com/science/article/abs/pii/S002231151930399X
RTE Number 1484