NSUF 16-812: Microstructural characterization of 23% burn-up MOX fuel

Attaining fundamental understanding of fuel performance requires detailed characterization of irradiated fuels under variety of irradiation conditions. Such characterization was previously limited by instrumentation available for highly radioactive samples. Significant advancements in understanding of irradiated fuel performance during irradiation started to occur with implementation of stat-of-the-art equipment in nuclear fuels field. The objective of the proposed research is to utilize such equipment to conduct detailed microstructural examination of the fuel pin with one of the highest burn-ups ever achieved in prototypic fast reactor fuel pins. The microstructure of high burn-up mixed oxide fuel with local burn-ups of 3.4-23.7% fissions per initial metal atom (FIMA) will be examined. The wide range of burn-ups present in these samples provides a unique opportunity for studying fuel performance throughout life. The high burn-up structure (HBS) formed in irradiated fuel will be examined in addition to the radial examination of the fuel pellet, which will be focused on understanding the effects of irradiation conditions on the local microstructure of the fuel. This RTE will focus on ACO-3 fuel sub-assembly, which achieved a peak burn-up for ~23% FIMA and a peak fast fluence of 38.9×10^22 n/cm^2 (E>0.1 MeV). The proposal will conduct microstructural characterization of the fuel using transmission electron microscopy (TEM) and focused ion beam (FIB) tomography. The acquired data will be reconstructed to produce 3D volume, which will then be used as an input to MARMOT.

Papildoma informacija

Laukas Reikšmė
Awarded Institution University of Florida
Embargo End Date 2026-02-27
Facility Tech Lead Alina Montrose, Gordon Kohse
NSUF Call FY 2017 RTE 1st Call
PI Riley Parrish
Project Member Dr. Jason Harp, Group Leader - Oak Ridge National Laboratory (https://orcid.org/0000-0002-5345-8440)
Project Member Professor Assel Aitkaliyeva, Assistant Professor - University of Florida (https://orcid.org/0000-0003-1481-6804)
Project Member Mr. Riley Parrish, Postdoctoral appointee - Sandia National Laboratories (https://orcid.org/0000-0002-3064-3862)
Project Notes Awarded on 12/16/2016
Project Type RTE
Publication Microstructural analysis of irradiated mixed oxide fuels Riley Parrish, Assel Aitkaliyeva, Jason Harp NuMat 2018 2018-10-14 - 2018-10-18
RTE Number 812