NSUF 24-5166: In-situ TEM study of irradiation effects in zirconium oxides

Zirconium alloys have been widely used as fuel cladding materials in light water nuclear reactors (LWR). In service, the inner cladding surfaces are progressively oxidized by oxygen containing species from the fuel pellets. The oxide layers formed on the inner cladding surface can degrade the thermal and mechanical properties of fuel rods and limit their lifetime, so it is important to understand their evolution under irradiation in order to improve the modelling of rod behavior in the reactor. In this project, we propose the use of in situ transmission electron microscopy (TEM) to conduct real-time investigations into the microstructural changes in zirconium oxides at various dose levels (0.5, 1, 10, and 20 dpa) and temperatures, specifically at 20°C, 360°C and 600°C (approximating the inner cladding surface temperature). This study aims to collect reliable data on radiation damage behavior in zirconium oxides, which includes the formation of defect clusters and the phase transformation between tetragonal/cubic-ZrO2 and monoclinic-ZrO2 at elevated temperatures and under different doses.

Додаткова інформація

Поле Значення
Awarded Institution University of Wisconsin-Madison
Embargo End Date 2026-07-01
Facility Tech Lead Wei-Ying Chen
Irradiation Facilities Intermediate Voltage Electron Microscopy (IVEM)-Tandem Facility
NSUF Call FY 2024 RTE 3rd Call
PI Junliang Liu
Project Member Dr. Wei-Ying Chen, Material Scientist - Argonne National Laboratory (https://orcid.org/0000-0002-6583-4204)
Project Member Professor Adrien Couet, Assistant Professor - University of Wisconsin (https://orcid.org/0000-0002-7330-5150)
Project Member Dr Junliang Liu, Assistant Professor - Florida State University (https://orcid.org/0000-0002-9278-6463)
Project Type RTE